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            ENGLISH| 武大主頁| 學院內網| 化院信箱
            學院新聞
            能源領域旗艦期刊《能源環境科學》發表肖麗/莊林課題組在CO2電解器研究的突破性進展
            來源: 作者: 更新時間:2019-05-27


                近日,英國皇家化學會能源領域旗艦期刊《能源環境科學》(Energy & Environmental Science,影響因子30+)在線發表了化學與分子科學學院肖麗/莊林課題組關于CO2電化學轉化的最新研究進展。

                將CO2轉化為液態燃料或高附加值化學品是近年來非常熱門的研究領域,其中電化學方法是最被看好的途徑,因為電化學可以直接利用太陽能、風能等可再生能源產生的電力。不過,電化學CO2還原這項技術的前景一直存在爭議,有研究者擔心CO2在水溶液中的溶解度低(約40 mmol/L),會限制此技術的工業應用規模。突破CO2溶解度限制須借助氣體擴散電極,特別是采用聚合物電解質(polymer electrolyte)代替傳統的液態電解質。然而,由于缺乏適用的高性能堿性聚合物電解質(APE),目前多數CO2電解器不得不采用流動電解液的設計。

                我院肖麗/莊林課題組在堿性聚電解質燃料電池(APEFC)方面開展了近二十年的研究,近年來在材料、催化和器件等方面不斷取得突破性進展(Nature Commun. 2019, 10, 1506Angew. Chem. Int. Ed. 2019, 58, 1442)。同時,他們積極探索將高性能APE應用于CO2電解器,終于取得重要突破。基于APECO2電解器工作在溫和條件下(室溫至90oC),采用純水操作,無須加入任何液態電解質。在60oC下,該電解器的電流密度高達500 mA/cm2 @ 3 V,與工業水電解的電流密度相當,而且CO2轉化為CO的法拉第效率達90%

            這是一項極具工業應用前景的研究成果。形象地講,使用一節鋰離子電池,便可實現CO2的工業級轉化。這一進展也將徹底打消工業界對CO2電化學轉化技術的顧慮,同時由于工作條件溫和(無須高溫高壓),技術成本可大幅降低。下一個研究目標是將CO2深度轉化為乙烯,以擺脫石油依賴。

                本論文的第一作者是博士生尹征磊和彭漢青,他們分別致力于CO2電解器和高性能APE的研究。


            全文鏈接:http://pubs.rsc.org/en/content/articlelanding/2019/EE/C9EE01204D




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